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Harolds Cross is a locality in the Queanbeyan–Palerang Regional Council, New South Wales, Australia. It is located about 11 km northeast of Captains Flat and 35 km southwest of Braidwood. At the 2016 census, it had a population of 53. It had a "half-time" school from 1868 and 1915; from 1949 to 1857, it operated as a "provisional school".